J, There are three more episodes I have seen Columbo display anger: "An Exercise In Fatality", "Mind Over Mayhem", and "Murder Under Glass". I will not spoil it by pointing them out unless you want me to.

Another is DEADY STATE OF MIND. I've never been fond of that line directed at Dr. Borden - "No, I'm asking YOU!"
All right, it isn't actually SHOUTED at her, but it is unpleasant. It's a little like the big moment between Columbo and Joan Hudson, but even less called for, since this person isn't some accomplice.

Grant, I meant the episode you mentioned instead of "Mind Over Mayhem". Sorry

That's understandable. I confuse those two titles constantly.